Table Of ContentREPORT DOCUMENTATION PAGE
ep ea ea TERT COVERED Fram TOT
Litigezoon Eaatiis
TEA STE a CONTRA HME
Electro” Aerarhmert and Jetwcbnent: C6? g
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CST ORERTCRTEN RE NE RSORESSES| “Fi Feo ORGANTZATONREPORT|
arch Laboratory
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SPORTS REPORT
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AORL-VS-AR-TR-2004 2098
“EES RTA VATA STRTENERT
Joneoved for public Releases Pisteiuecton malisiret
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TOMETEO PEE) PHRNRIZSRZS GQURNAL, OF UASS SPECHROWTRY, Vol 232, up 67-73, 2008
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‘talus be ase e298 asa das i. He expel che OED eee god wide 916%.
Batre BA At igheneened
5 ORRET TERS
Elgeron olieschnant Riecuecn detachrest Blecten affinity
Hoxaf Iuorobensenc
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REPORT BABS [= vifapnae | san 7 2 PE ER aS
mass mes waa Faleav7-4028
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amenee Goinsore
Electron attachment and detachment: CoP
‘Thomas M, Miller, Jane M. Van Doren", A.A. Viggiano™!
sab time Rag iss es sae oe i fo a bo A 0
Aen
Lester sneha nC ely ses bem of eg hana aay tao he nm Dy} od wou >
‘Wethemaie acts come ecm us lye esa eer dese a pan CaS
Dirthtonpeomremnge 397 ALOK ia 123i pe A Awingentbgr c EALP ape a ai uA
Bee thee ran coe le BBESD TD +a he Geb mst apne 31 A
the ena inceases ty eres pi 200 ta 4, Te ceecncan ele ta ages ha i eon
Mcp egh hos} L 9050 Det Seta eens ne coe tc wo ec Be eae nda aoe Lb
oie uur hi es TGP, COPD aan ye meron nye M44. Te aii OCP
lend fete La6e¥ 398% wg thc ue in, No cep Ps CPA rales be gen MIME. Ce
(Bien Phen Adrien
1 Introdostion
Hexaumbeneene (Cilz} tn an sletestng and cor
walnut tnsegad tb fonnatio fe pre en
Sn goes An ely tem ros peter reset
bth elec ally eave EACCGFa) = 184 0508 1,
nd ths rest mislead ater exeruoeues Ue
Toor seein acer rt lead agen
tat. To mals mares wore, extents conse
gest ler pla RAC) > He Band <1 Be PL
fn 1984 Adams tal. [3] m8 Spsvon nd Cristp ua >]
seve hat age to ean Gipscedoned and dr
tao devceee i the ate colin Kr eecnw cheno
Uo Cat will enporaae which would imply a aezuite
Caphysia actain ney feet sche
"a 16 hen exphsined 1 comuncra By pit ot
fle uainod a about the same tne a elecen ee
fete: Calg ws they deching the wer elton
at clevied pera, ar & te tar implied EA of
0.5 008eV TF Tis explain was wt innately
lcm ago)
139-3 «we mnie 9 2 these Ae
scceged SL, snl becuse of te scomingy igh EA of
(akon cnsiaing tho ne vale of 08629.
Stony wheroor, ia 19R6, Chewdhury et sl wed
igh posure nae spetoriey to menses) ad
feand 032-=0.202¥ 9-1 Jal wed Gar tal tele
nent womb ike plate a det expertps. In 1392,
Enighon etal. [12] contiml br eke descent
cpio at povnge sxpetiment nd este ue
nets fete dealer protes user Be tarsal
ange 307-349 Much of he Kaighen etal war regrded
ths cof woateabe oxygen igen Ph presets
experiment hey etclaed tar pressor: exo
tstrind eu woes spetmiacircaalec e n,
sh ab the nf Syme an Cheogveu (5) and Chen
fal [ewer anlely to be omer onze. Iv 3
face wok, restos belseen Oz” and Cy ere found
te be eoliseual and led & fagmontnin of the Cin
{Ds of he recone renting mee ste Ch po
cet [F9| Renton helowen CyPy~ and Oy ee 50 dee
Somer apd led © tral arangement of he react [3
Tae sry Bos ter ere 1998, Chen 6a 18] ro
pul the CF cleo capt deters exeroest ot
tained ES(Cyfeh = 03-4 1226 fon Maseasared
Caton ion sign, Ta 1995, Chisophoran and Dashes
TS wed dhe te seslve eee rn sia ih
« 7H ins at hana aa en ENE BOO
gh presse of Ne ber gas 10 meso at costs
far bath etn lsh Cg an detachment rm
"a ea cleeuon eneegies fre 02 :e €0CY ood
tempenities Fo Tre STSK. An Abe pl fhe
Aeuchwen ae const yieled aa aston ectey of
‘Oa772V, which wae ken ay a estate of EAICAT)
‘cand dar ame tne, Kikai e al reports! pA
lecton energy yes Fo Che” hich they erp
Ub gting FACS Fpy © O80:4910e¥ [16], Reco, Chon
find Chon {171 ive inesrted ele ere deste
‘ete eing toeeecerie sae of CoP, Whee
tron fing seen of 80, G70, aml OS5eN. Tose,
[Sail yor [14,19] 0 NO and Op fo Chen's Lo
Tey Sie in foe of velba spececeropc
sks al 6 clary ong. ‘Thin point has been fre
Tally mee ty Bevo e 19D), tin enlided dr a
‘cctto captive deelurtaswlenets of clstron ahi
tps shell he coevened sujet tage and wok
"We have cule i th “sts he eoromor: compet
ce aur tance that he oars CaP atc
Jive eon in an enced sate, an hjtion ainda ay
capri supporting sls val of EAC) (bu
‘Seedy he eosin, seers el al of De
fxgesiol Be buler gry sure 84s Mig eno: ht
{heals and another they werent te
sal eit he halo gas. The sing afew
Tegan probe (FALE) expaciment cept Pere an
cf Adare ofS ceme o low prsute He 3s
ti wats cla along tis ne [2U1, Pte PALE ese
fave ben oonscely ford iver wih seco,
gue nas 27}. che ga pry ear aan heen
rods face ie nner ad, he
fei concentration gamely 30 fiona
Teaiins enol a raie he wanespacear. oat tere
{bee rporing hese sus fr elecron starches Ce
ad dchmert or Cau the npn in re
UEEACCGES). Asbo in Ret [3 ale vom ele
tron denn co ill on Aarsnio bavi,
Ti the pressnt work, we wil Zccant for entopy emg
Toviding the imprinted ney ae, ae
the fntegead apcii has of Cay ed GP, in Deter
mining BA‘CsFy,Futeomere, we famed an ese
Fanta and CMPD) calelaons of EAC)
“The clecron-heam expires of IngSifsoo ul Le
tegee24lireilreting murdering ston zh
ra gy bosene dy swe as one meg eess trom,
"he thermal eeperrien tha Ieee Rs aE
[Shute aro eoogy sane, ging eet pte
ino ovleyeenced Paluch xan sale te ao,
inthe ection. To econ enemy hen een Wp
by ermal ede: ofthe Ca ian olf rindachinent
Iban encugh fortalitne oclisions Webitzation Atel
too sonics well sve those worse i rel apr
rent lesion Bea experimen coda ie opening
st endotiemie dsoectve tachment mets,
2 xpevimenial method
VALE aarims wan wel for is ode ar be Ac
once Reveth Laboratory. Beth the meted (25 al His
Duvet gorau [26] base been me dca a Bo
Tewtae at wil nc be detailed tee, Tae easements
pete cid out in 152s eps Tho CoP 20s 27 5
inreduod ioe te fom be a3 cones of ply
4a0ypby. Ao eel ul The data ohaied is shown ih
Tig ts such a tse sere Atte deen dh cleeon
atthent const an th dace rato conatt
fe Ths reat each wenerate a given in Take T= 8t
the se tng, me ease De -achient at censtct
fir Sf a1 798K and ataned 226 10°F aes wich
skvse whe ateutte ve 227. UU 3 10-F eae
‘M1294 D2.
‘Se ie Rt (29), and eatin phe ee
ey deny ple is thus af ar clecven-deaching
pimas stem fie cine teaches 2 éifsion tui
‘Henly sate oadtinn et lng Hes The erly prc af Ge
‘octom deat curve is conta hy by. Th kel of he
Jake prt ofthe cuss edad By he Zn fh.
‘he enna epee dor deeming tha fer
“phish he atncboen!foueny oy = Ayre compe
fn rigatad to Ag (bth I ups of 27, bu ae han
“he amigo eon dy toa wy he Taner being
revs in yee of estat gs, eerste he pass
ftvas kay hefee the sete eli yeaa
‘des fp ae sald Jab for cormaion hy
{ses of ay vey Tn itecet experiments bees A
{he amulet of Ar o> ee toe A) We noe at
{heel a dependent or ce sense vates of he eae
tram dency a ong at et elasion mab deat
SeRoeE
t
: :
E10 Later aia
An meet Ab i rie yo 36
UE te a sin sf ee Spe 2 (EH
ses eC an te
TE ue wee
Bam cmos te non ain mu te se
{abe roan po such eal then te eactant con
eaton That i, chapiog the ini lca dees
ingly moves the curve ia Tig. twp orn a doe a
hangs haps Ff, be a tbs ess Fe
4g ae iodepeoeat of m, since by is a wilt rat
SOIR 18e CyFy eke these eonederains ao that
St 2OEK the da Sve ke acaraly bit wot a By TDK,
fe apps ths same magatade sp. sing Te
lecwan decay curse an exponrotil wpesvnce ws eee
fr detach ons wr sane de fe fife, AL
Fighortrperutre, tie eve Jaks fa Tig 1. At il
Pither temper here is much reir tan Be
clecwon density cure is atl indisingustble from
The anin cure heme ow CaP acess Me 50
rush ee ney dar the 2a elec eat eA
‘Maca iengh ukave any elit on de elston
fecsity At 400K, we aust wee such ih eoncecatine
If she 8x INcpr1 a he seat conde
teveed $a ah a short eae that Boers iti fe
Cierine lf soca ln
test uy Be studiod mth he FALP appar only over
OSE teepentue ng.
"We have etic given te st of obtiing te EA of
he etn om heel cunt if 29) The
‘equiv costar yields he res energy, SO*-T obtcn
Te alge Ath, te ergy oF ret nes be kas
“Them he EA my he obtained by wing igre beat et
finest educe AP vp dhe metas tempera T
OOK The neces ectopin ane sgt bet cag
(eet le easwed,etonred of calenned. Th effet
I-omaly noc ges ee of Vb sic
fn detemunng At which ac cry ame bode of me¥.
Tie D5). mde severest otain ex
troies uo integral sects Hea. Size then, Re
feo ribo routinely cals the neve emetins
[22] sid hos prose a mue asta ae forthe EA of
the rectn
5 Computation et and esl.
“The G3QMP2) raed 130] sv aged 0 CES and
(Cay in ander to cbt BALCH) For comparison with
lie expert ule The tod is aca ox average
Seth SGunV for alge txt set of moles of a=
ately fac press (30) Ton expe, i xe
fe he GBPS) A tobe wrong yee 10°
TBE, Density nto thon (DFT) ws apie ese
holes sonar cht: enuozy and beat capacity Ue.
tides oreed 1 xeevty wera FAL? daa in ms
[oF WACsfa) DFT export tn provide tase quates
ote ancuately ti de re-take) thd Ral
into the USB?) preanition haan cloeuon cocelion
Ie approximartyatcounte fr in he DI Sines and
ecu a igor baie wet ay be used than is spied
Ih the BF petinn of the GMP2) reserpine the
DET BAS ten tobe 02-056¥ to igh €eoting che
bass set cel. The Cant O9W pong package we
‘ied forth the G2NMP2) and DFT werk decid bee
122), Toe sbi of he Seton use was ccd
in eich gan, te. it an vere tthe motel cia
‘et ebver el ote lowe nergy watefunton,
‘Te GACP2| Frain 305 tho HF eho te obin
zero-pinc energies ZED) on ee ery mljunens
Crevbalhiet and hee entgce. wth harmon voraton]
fequeeis sald by OB529, High tevel eneny ell
tions eee on AOC Det geometry abana
ing sscond onder Mises perurhason hear (MP2)
sei ie BTC hala anal lecus. As cecsinally
hsp wing eho GR cts. the HF geomet fer Ca
tas ess gmt thn deste MP2 say 99 the ZPE
faethe aon fe ot evel cones, bt en diferentes in
the 20% ene the FA(C}4) reu. The DET calelaons
leit tthe ZPE sue tects ECA ate Tice
level thei hve! (MI ealulation wee cai ent
fev Thg, CgFa and Co, CAFR afer he MPZVG-S1GIC
Span pms a se cas
“The DUT catenins were prt singh LY
hyd acconal 3] and he 314330 beet
CCaewted aroonic sibeaooalteyveciey oer se
hy O49 [25] copies Gath rckeaarspmnccsgtza
” a ie ivan ama iSpy 2 HG 28
en a Mets yt cf CA Phy lt ae FA
cos cose ber
oe or ee com
BBE ne aa het ite
Bar ase " roa .
eee to te im
aoe eo as ue
rein En Tea Sg an pe ha PRGA OS
ERE Can be ny cnt ny 00. ae GeO Pon LS 46530 Yd a an ey 939, HE ea
‘ptt main ad BD Ioan als 2 er TET
above anime ent eaecies wero calieted a eh
Tenpercu for which cele fy rte cosa were ob
fan. Vales cll at 350% ao included iTable 2
bong oh tal enevgice abt severl peomeby preter
“Tg ot shea exp nae 2 ean ta Oe
‘ional erry chee etcen Cay and Calg shat
‘gsr tan he eotionenipy cheap esc ih
‘hs lage chung ny atin syne meer. The DI
TEACCgE) i als gion in The 2, Ua eapvionss has
boon tat vl be (L252 1b Bl Forte Bs St ws
ere [36-A hough sad of DPT mths ir dt
ing EAs bas been poster y Wins Kafe ea [7
vows (Fy is cbiouny completely plats i De,
sym, Toe ms sible Fst th ealeuled mica
Secure tat (nono ams a pst. 1 and
22 pod abv the merge carom ple hy ahowt 2
{Toe C worn tn whic ese tn F aoa ape bl he
‘eyo Blew dhe pane in wich the ean four
(.2. 3,5) of 0. The
es an ie plano to, lily
Flow that fie fone pana as ions, 5,208
6) Sven tne leva omer] peacters me ser a
Tetledand the Cslq_ secures shown in Rg. 2 Tho HE
suc ot CaF ha the Fst at psion 1 rong
fee ou ott verge chon plane han the Fae a
poster
“The Cy anon rte yen hee Sonten wi at
elena 39 seu ago Soregalevy ot a [92 ah
{Ea eaeley Feceks oa 9) 8 Trea at
‘luca Tv a8 ESR epeezun 40) as cece in Wa:
cr
The GMD} energy of CAE" wy calelansd
(M6 56807hereee at UK ad 93655044 bacwoe at
208, fiom whieh abs the ede ity nl CO
24a OK} or 2heW G9EK. Those wales ae =
weet: ec pm Tobe Fae pcs ope
sonable agement wih she experimen resto Mizu
ra 44 1264 ico uncertain phen
4, Dicwsdon
“We nore tthe symmetry change horbecn CaF aad
Cafe Sys porte ne chm
pees: Neural CGE has Dry prey (iD a ection]
pron mune af 12) whe Ge anion hs Co genres
(uit a eatioal symmetry see of 2). Eis degree of
songe hs higi'y nos and the conan es 1 ie
fEntggy change fo elcror staccato he
‘sonversun fra a eared equi coat a BA
Sas Aother yf hag Mio su that ese
were change in Symmioey Betren Cay ad Cate
{he detcten rte oon sual be 36 ties gee han
sere at 1ST!
4st st tsi af Sms 2120S ”
sfeson eaters creat
Fig 3 A worn den Sache fcc bf Cs
Set
The weaured h sabe QO 20 » 30 Mans? a
298 ils sgl bm han toe ese Ada
al fH sig the tame meted they oboe 1.22»
orem 1 3ONE, Spo sal Cannon [5] oo
ea omar ala cdr estmeanclectam nergy af
‘Base al gas temperance oF 00K, mt bigh res oF
1p Atcaning Whe ela ear nel of Kes FE)
thi A pesca about one negate ian fred in evry
ttre clu bln Cy at lin
Tai. 3 ae prsent es or (oti n 13a
ss} tanpaval tho Rego: tal [12] oknaed
2 GTR CH gn tone of Cheon ant Darke
#15] (lmined in $0 SOD¥PGN; ge) The Iter e515]
forespend to mean elccon egies ate 00% bl the
tonne appear oe indeaden 0 eeu00 HEY
therange 020-0380
Ds sr Re [79 ey fevered
pendence sien by
to)
ol -(8)-(22)-Cat))
&
‘The leew paths ey ten AS” in dhs a-pomen:
of hs exponen combs & fcr of Fhe
Tending vormertre dependences #2 a (Nk
is Belmar’ cao, Zi Lech aumbet, Bis
the elon aint oF Cal a DK, hy defaion) AF 6
Theenttopy change dus telecon tachment, and By —
fa he feral eney eres one tue Ihe PA
resltes OK. The Tespendensecf fy ith completed by
Ua cmt ply her nen sh 3
ho beat epsces ofthe noua and anism To ee pen:
ve Ganges sey lle Ue nave ere ae
seceisle es.
EACala) say be obtained fom the mised by and
saosin he iva ot Eg 1, th de ion it Re,
[Bo] fa eras of AG at AV”. An ample wl be given
far the 30K dita sige erage lus rum Tale
OF UAE Oey apd Ay = MOS The
RATYPGALEGGR) De exculaion yoked canepy
nd Stealers copay sles for Da, Cas and Cas
Gabor ven in Tah 2 Th entupy ching
siason) ~ Strout ~ Sshetoe, ©
AS =4686— 4228-0281 KTANOK
fora nec como cbrage of 207 me” K+ The ered
eat enpcties ela contedhe"EAT at S501 a Uve
Fagarok) are
arate feseeammar f someanar
[comioner ®
By = ya TS 4 AS — STG na aE, %
‘heinoshemical quanti forthe ehetme a expec
wing Bekoroamn sts fren Td out in ie JANA
‘ables [87] The nar change fm itgrted heat capacity
‘Sonat 380K. The Sal eeu ong tee oes
By {0 & EAGHGi = SEne Ott Bemetbercal
ance nth se umes are A" = Me at
Bar = ~367 meV 9 ASC) Sir anal efda or
‘whish opimam sation: okay, separable Ay ad
Tul ger Ban dp) si wan aveage vale BACCaN)
(540 Os re. The uncertainty i cee byline
Fowl fy ake sine vlc ad inlingadinal et
fied unsenang fate keermize rel viral a
pusible ers the esevared enrng and het expt
ijustine BA ls ony a ogarthic depsolerce
fn heat of ftp yy BA sae Soest es
fr dhese uit, Accuracy i the penne cei
Poet ie portant, buts ssi atin ors ath
‘alte enlegres on pate Hea capscin aos BA
Eth fastncoFaac¥ lve Te et he seen oe
‘euapate gre, DF sr eaedaies fF, OFS,
fad 8% re corgarcd to thor inthe JAKAT wes 3).
Geral pening ve ound tht fe ng te lal,
Thee the green ecwete DIFC ad IANAE. Pe SF,
the cloud enon results ae good win 2% ia the
temperate range te een ei a the seule =
repre eat capacity agro din 9%, Oaly iferences
‘etvesa newt un adem enupies siege ht ce
ucts cee Im the poset HA deerme, and these
‘rence moun a Heh cbr individ ats anon,
Teen se esl alloxan oely aoe 1%. Fur
‘thermore, case alse nue ly SH he BA,
salve Tn, atcotaiin In dhe alowed eral djs
‘ent are eelibefsohe us EAC) is cone.
» YM ier ans am Spt 28 0S
omc hope BA, Deny vals eneusod wing st EA
are outemr’y serve hacuraey MEA, In Te. 35 the
tise ns ae evahious of Ex (1) rch case oop
ice ie thee lab gaa es Tine passing oO
(he peseat /ALRIj ale ue BA = S2Dme¥ Hat for Be
‘ORNL 15] es BA = 48402 alt fre IST
fh (2) ones BA = SO7rme¥. AI ce lings ere ale
Tak sing eu 298K val oF, 8.6 6 10-Fems | ae
tie nd est epee celal wing deni Fane
{onal tory, Teese entries and Bea eapocis oof
‘nse, lenge depend, bute et ele thea
tne ofthe exponen in (3) changes BY onl FeV
ver he JOD-S7S rane oe drain Fa. 3M the ti
{Ee ORNL nd A da ee pubic te ln
civil uf of LO. LO"Fam =e asaes ths dat Te
‘esl he dated ees tn Hie i ger salve
(Fhe te EA valent baie sigh by 0a Hoe
{RN dy 3 me fer MAST a) a oder ke he
Tse pte rough the ceil of he specs dat se
Altlthoncaypurct BA values are whine 10m a
‘etait eetinse fv the SAD-ne a ded fom te
ren rchrcilSuchien! expec
“Tosi, respect sal peaking eases
AG? at eah tomers, The terrain ut HACE)
depends on earopy and eae, quanes which ast
‘enue eaetere. The envepy na eral het capa
ig for he leon are svat ie allan sates
HSL. Teeny and itd het expat CaF
fe APG partly coool excep or ie kaon efoto
Secon pi deyensney aol toatina sari manbet
‘The quate sabcaet wing DTT irtics 434 meV i
provement wor a ne WOU eine witout Ie el
fed quanies, uc vas dour i Het 28). Teal
dn th eternal guns aoc the BA. deeiten
olay tee lve, sot is appropsinte w easier oar
TAK) Ht 1 15e¥ tse aap cxgesinat oe.
5, Condadeus
‘We lave made meabuoen of rite consis See
tron atachment Cle ant ernal loaton dexasint
Hom sh parent anon. Py. over Le enpecare te
294-40 Kan (31Pa n He pae In an PALP appa
‘Ac 208%, the eoedon atashnest rue msi Ay
630% 10 Pen? | and ihe daaslent ae comet
Igisepnoxinataly 357) Thi dae alii over
i recs [4S at face win
Tite Ae te spore nesses iy teases pi
a vale of aboot 30008 a 4006 "The lng chang
‘pintany eteN Cy and CAPe, fmt Da, fo Ca,
fang ta surprest th detache proces frm wha one
seo gu ae le the a lero af. The
sacuncstetchnes equ pes ht he eer
nity ut C3¥, S24 OMEN. eit funetoal ale
Taine were cai nto ors abn eatopies wn hat
apa acodi 0 conve! te egibum eos
in EAC) hue nel GME enka glk
im leon ainy of 0434 on 3 Mee tty fa
aR ol L2GeN a EK. tn ut experience, the GACH)
revue ae oe rn 1
‘Note ated In root
hie this publi wae in pes a through here
ics sty ofthe gh ion peared FA si apis
tele psc pochsone regard i a, 2) 3
‘ths enon, We stoul sss tenn she pe adilss
ey of elocman sachet CaF to 144 Xe by Th
‘Shimane ta:
‘Acknamtedgements
We dotiite thie work to our tind Prot De. Tan
Duk Our pis loosed often wid elem att
puncte a8 eonfcenes er letrsip the pre
fie lon Phys nla atthe Unnesy ofIresrack as
some an inspiny pice 0 vs
‘We ae wate oe spo ef be Ait Force nen af
“site Rea for hz wurk IMD. was a Natens]
Acne uf Seinces Seni ising Floyd ete
Fh TSCM. undercoat 98D 99 C0060)
‘ih Viiyae Tne, Dealing, MA, USA,
(me at, Men, A. ae Cha 9192
RE ae-e sh A te, Chem: LA
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