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O ,. 0RNL--6 086/VI DE91 000527 Physics Division ATOMIC DATA FOR FUSION VOLUME 1 COLLISIONS OF H, H2,He and Li ATOMS and IONS ' with ATOMS and MOLECULES C. F. Barnett Oak Ridge National Laboratory Published and Ed,]ted by Controlled Fusion Atomic Data Center O H.T. Hunter and M. I. Kirkpatrick Series Technical Editors I. Alvarez, C. Cisneros, University of Mexico, , and R. A. Phaneuf Contributing Editors Date Published- July 1990 Prepared for the Office of Fusion Energy U.S. Department of Energy Washington, DC 20545 Budget Activity No. AT 05 30 04 0 Prepared by the OAK RIDGE NATIONAL LABORATORY Oak Ridge, Tennessee 37831-6372 operated by 'MARTIN MARIETTA ENERGY SYSTEMS, INC. for the U. S. DEPARTMENT OF ENERGY under contract DE-AC05-84OR21400 _ _ '_i ......r. Printed in the United States of America. Available from National Technical Information Service U.S. Department of Commerce 5285 Port Royal Road, Springfield, Virginia 22161 NTIS pr=ce codes--Printed Copy: A-99Microfiche A0] This reportwas preparedasanaccountofworksponsored byanagencyofthe UnitedStatesGovernment.NeithertheUnitedStatesGovernmentnoranyagency thereof, noranyof theiremployees,makesanywarranty,expressorimplied,or qlF assumesany legalliabilityorresponsibilityforthe accuracy,completeness,or usefulness of any information, apparatus, product, or processdisclosed, or representsthatitsusewouldnotinfringeprivatelyownedrights.Referenceherein toanyspeclflccommercialproduct,process,orservicebytradename,trademark, manufacturer, or otherwise, does not necessarily constitute or imply its endorsement,recommendation,orfavoringbytheUnitedStatesGovernmentor anyagencythereof.Theviewsandopinionsofauthorsexpressedhereindonot necessarilystateorreflectthoseoftheUnited StatesGovernmentoranyagency thereof. I iii ATOMIC DATA FOR FUSION VOL. 1 COLLISIONS OF H, li2, }le, AND bi ATOMS AND IONS WITH ATOMS AND MOLECULES Foreword ........................... xiil Series Preface ........................ xv Abstract ............................ xvli Introduction .......................... I-i A. Electron Capture Collisions H + H -> H- + H+ ........................ A-2 H + H2 -> H"_ + H2. ....................... A-8 • . A-10 H + He -> H- + He+ • ..................... H + Li -> H- + Li+ ....................... A-16 H + H- -> H- + H ........................ A-20 H. + H -> H + H. ........................ A-22 H. + H2 -> H .......................... A-28 H* + H2 -> H- . ......................... A-30 H_ + He -> H + He. ....................... A-32 H. + He -> H- + He2+ ....................... A-38 H. + Li -> H + Li. .............. ......... A-40 A-44 @ H. + H- -> H- + H. ..................... H_ + H- -> 2H ........................... A-46 H* + He + -> o(He 2. Total) ................. A-48 H. + }le. -> H + He2_ ..................... A-54 H2+ + H -> H2 + H+ ....................... A-58 H2+ + H2 _> H2 . . . ...................... A-58 I]2+ + He -.> H2 4 He+ ......... .............. • A-58 H2.(u) + H2 _> H2 .... ..................... A-60 He. + H -> He + H+ ....................... A-62 He+ + H--> He + H ....................... A-86 He. + H2 -> He .......................... A-68 He. + He -> He + He+ ...................... A-70 He. + Li -> He 4 Li. . . . : .................. A-76 He. + He* -> He + He2* ..................... A-86 He2. + He+ -> He* + He2+(Partial & Total) ............ A-84 He2. + H- -> He. + H ..................... A-86 He2. + H -> He+ + H. ............... ....... A-88 He2+ 4 H2 -> He. . . . .................. A-94 He2* + H2 -> He ......................... A-96 He2. + He -> He. 4 He + ...................... A-98 He2+ + He -> He + He2+ . .................... A-J04 He2. + Li -> He+ + Li_ ..................... A-I10 He2_ + Li -> }le + Li2. ..................... A-I14 l iv q B. Electron Capture into Excited States Q H_ + H -> H(2s) + H+ ............... ........ B-2 H* + H -> H(2p) + H' • ................. B-8 H+ + H2 -> H 2_) .................... B-14 H. + H2 -> H 2p) ..................... B-14 H. + H2 -> H Lyman-a Total) .............. B-16 H. + H2 -> H Balmer-_) ................. B-18 H+ + H2 -> H Balmer-B) ................ B-18 H. + H2 -> H 3s) ..................... B-20 H* + H2 -> H 3p) ...................... B-20 H. + H2 -> H 3d) . • ................... B-20 H+ + He -> H 2s) + He* ................... B-22 H* + He-> H 2p) + He' B-28 H. + He -> H Balmer-_) + He + B-34 H. + He -> H 3s) 4 He* .................... B-40 H. + He -> H(3p) + He" • ................. B-46 H* + He -> H(3d) + He+ .................. B-52 H+ + [ai -> H(2s) + bi+ • ................. B-58 H+ + bi -> H(2p) + Li* • ................. B-58 H+ + Li -> H(3s) + Li* .................. B-60 H+ 4 Li -> H(3p) + Li_ .................. B-60 H. + Li -> H(3d) + Li+ .................. B-60 He+ + H2 -> H(21S + 23S) .................. B-62 He. + H2-> He(21P) ...................... B-64 He+ + H2 -> He(31p) ...................... B-64 He+ 4 H2 -> He[x = 44"7.1 nra) ................ B-66 He+ + H2 -> He(x = 587.6 nra) ............... B-66 He+ + H2 -> He(x = 667.8 nra) ................ B-66 He* 4 He -> He(21S 4 23S) + He+ .............. B-68 He+ _ He -> He(21p) + He+ ................. B-74 He+ + He -> He(31S) + He* • ................ B-80 He+ + He -> He(31p) + He" • ................. B-80 He+ + He -> He(31D) + He+ ................. B-80 He_ + h3 -> He(33S) + He* • ................. B-82 He* + He -> He(33p) + He+ .................. B-82 He+ + He -> He(33D) + He* • .................. B-82 He. + He -> He(41S) + He+ .................... B-84 He* + He -> He(41P) + He_ • .................. B-84 He+ + He -> He(41D) + He4 ................... B-84 He+ + He -> He(43S) + He+ • .................. B-86 He+ + He -> He(43p) + He' • ............... B-86 He+ + He -> He(43D) + He" • • ................. B-86 He+ + Li -> He(53.7 nm) + Li+ ................ B-88 He+ + Li -> He(58.4 l_n) + Li+ .................. B-88 He2+ + H -> He_(2s) + H* .................. B-90 He2. + H -> He+(2p) + H* • ................ B-96 He2+ + H .-> He_(Ly1_lan-a) + H+ • ................ B-lO2 He2+ + H-> He.(Lyman-B) + H_ • ................ B-lO2 He2+ + H -> He+(L_allan-_') + H+ ................. B-J02 He2. + H-> He.(Balmer-a) + H_ ................ B-J02 He2. + H -> He+(3p) + H. He2_ + H -> He+(3s+3d) + H*................................... BB--110044 He2+ + H -> He.(4p) + H. ................ _ . . B-104 He2+ + H2 -> He+(2s) ....... .............. B-J06 He2+ + H2 -> He.(2p) ..................... B-lO6 He2* + H2-> He.(LY man-=) ...... '. ............ B-lO8 He2+ + H2-> He+(b_.an-B) ................... B-lO8 I V O B. Electron Capture into Excited States (Cont'd] He2. + H2 -> He+(Ly111an-Y) .......... . ........... B-IO8 He2+ + H2 -> He+(Balnler-a) . . . B--108 He2. + H2 -> He+(3p) ................... . . B-IlO He2+ + H2 -> He_(3s+3d) . . . . ........... B-IlO He2. + H2 -> He+(4p) ....................... B-IlO He2+ + He -> He+(2s) + He+ ................ , B-112 He2+ + i,i -> He+(2p) + [si+ . ................. B-.II8 He2+ + [,i-> He+(3p) + bi+ ...... .... . . . ....... B-I18 He2. + Li -> He+(4p) + Li! . . .......... . . . . B-118 He2+ + bi -> He+(3s+3d) + Li+ . . ., .............. B-II8 He2. + bi -> He+(4S+4d) + Li_ .................. B-II8 He2+ + Li -> He+(Ly_llan-a) + 5i+ ............. . . . . B'I20 He2. + Li -> He+(b]nllan-B) + Li. ........... ..... B-120 He2. + Li -> He+(by]llan-7) + Li_ ................. B-120 He2+ + Li -> He+(Salnler-_) + bi+ . ...... ........... B-122 Hez+ + Li -> He+(Ba].mer-_]) _• Li. . ............. . . . B-122 He2+ + 5i -> He+(Ballner-1) + Li+ . .... ............ B-122 He2. + Li -> He+(Ba]nler-o) + Li+ . . . ........ . . B-122 C. E×citatiol ! and Spectral bine Emission H + H-> H(2s) .... ...................... eZ2 -> H(2p) ......................... C-2 -> H(3s) .......................... C-4 -> H(3p) ............. . . ........... C-4 -> H(3d) ....................... C-4 O -> H(Balnler-a) ...................... C-4 H + H2 -> H(2s) [projectile ] .................. C-6 -> H(2p) [projectile] .... .......... C-6 -> (2s) [target] . . ................. . . C-6 -> (2p) [target] ............. ......... C-6 -> (L_nan-a) .... .............. C-8 -->> HH((33sp)+3d i ......................................... ....... " ' CC--1l0O -> H(Balmer-_) ...................... C- 12 -> H(4s) . ................... .... (i!-14 -> H(4p+4d) ...................... C-14 -> H(Balmer-8) ........................ C-14 H(2s) + H2 -> H(b_allan-a) ..... . . .... .... . . C-16 -> H(3s) ....................... C-18 -> H(Bahner-c,) .................. C-18 H(2s) + He -> H(L_allan-¢,) ........ ............ C-20 -> H(3s) . . . .................... C-22 -> H(Balnler-a) ..................... C-22 H + He -> H(h_nnan-a) ...................... C-24 -> H(2s) ..... ................... C-30 -> H(2p) ..... . ................. C-30 -> H(3s) ..................... <:-32 -> H(3p) .... ..... . .......... C-32 -> H(3d) ....... ............... C-32 -> H(3p43di .................... C-32 -> H(Balnler-a) ................... C-34 --> H(Balmei-_) ................... C-34 ~> H(4s) .................. .... C-36 -> He(31P) ...................... C-38 O -> H(4p+4d) ...................... C-36 ! vi C. Excitation and Spectral Lille Eluissio,l (Cont'dl. O H + He -> He(33P) .......... . • .......... . • C-38 -> He(33D) .................. C-38 -> He(41S) ........................ C-40 -> He(41p) ...... : ................. C-40 -> He(41D) ....................... C-40 -> He(43S) ........................ C-42 -> He(43P) ..... . ........... ........ C-42 -> He (43D) .......................... C-42 i H_ + H -> H(2B) ......... .............. .... C-44 -> Ii(2p) ......................... U-44 -> H(n=2) ........................ C-48 -> H(n=3 ) ......... .... ........ C-48 -> H(n=4) ......................... C-48 H. + H2 -> H+ + H(2B) + H ........... _ ....... C-50 -> H. + H(2p) + H ................... C-50 -> H+ + H(3p) + H .................... C-52 -> [_(Lyman- a) ..................... C-54 -> H(Balnler-_) .................... C-56 -> H(Balmer-D) .................... C-56 -> H(Balmer-x) .................... C-56J -> H2(L]allan-Band ) .................... C-58 -> H2(U_llan-Band ) .................... C-58 H+ + He -> He(21S) ....................... C-60 -> He(21p) ..................... C-60 , . . ................ C-60 -->> HHee((2311SS) + 2.1.P.'.)........'............ C-66 O -> He(31p) ....................... C-66 -> He(31D) ....................... C-66 -> He(41S) ..................... C-68 -> He(41P) ....................... C-68 -> He(41D) ....................... C-68 -> v.u.v. (20-140 nra) .................. C-70 He+ + H -> H(n=2) ........................ C-72 -> H(2s) ........................ C-74 -> H(2p) ....................... C-74 He+ + H2 -> H(b]allan-a) ..................... (;-78 -> H(L_allan-B) .................... C-78 I -> H(Balmer-a) ..................... C-80 -> H(Balmer-B) . .................. C-80 -> H(2B) ..... .................. C-82 -> H(2p) ...................... C-82 -> H(3B) ..................... C-84 -> H(3p) • ...................... C-84 -> He+(2s) ...................... (]-86 He+ 4 He -> He(21S) [target] ................. C-88 -> He(21p) [ta,rget ] ............... C-88 -> He(23S) [ta,cIet] ............... C-90 -> He(23P) [target] ............ C-90 -> He(31S) target] ............. C-92 -> He(31p) target] ............ C-92 -> He(31D) target] .............. (?-92 -> Iie(33S) ta£_get ] ........... C-94 -->> HHee((33]3PD)) ttaarrggeett]] ...................... CC--9-494 O i I vii c. Excitation and Spectral Line Emission (Co[_t'd) He+ + He -> H_(41S) [target] .................. C-96 _> He[41p) itarget ] .................. C-96 -> He(_iD) [target] ................. C-96 -> He(4]S) [target] .................. C-98 -> He(43p) [target] .................. C-98 -> He(43D) [target] .................. C-98 -.> He* (n=2) [projectile] ................ C-100 -> He+ (n=3) [projectile ] ................ C-I02 He + H2 --> H(Balmer-_,) ..................... C--I04 -> H(Balmer-B) ..................... C-]04 He + He _> He(21S) ....................... C-I06 _> He(21p) ....................... C-]06 _> He(31p) ..... .................. C-I08 _> He(31D) ...................... C-!08 _> He(33p) ...................... C-I08 _> He(33D) ........................ C-i08 41S) ....................... C-110 -->> HHee((4 _P) ........... ............. C-II0 _> He(43S) ........................ C-I12 _> He(43p) ...................... C-I12 _> He(2s 2 IS) ...................... C-I14 _> He(2s2p3p) ...................... C-I14 _> He(2p 2 ID) ...................... C-I14 _> He(2s2plp) ..................... C-]14 _> He-(is2s 2 2S) .................... C-I14 He2_ + H -> H(2s) ....................... C-i16 -_ H(2p) ........................ C-I16 He(23S) + He(llS) -> He(31p) + He ............... C-I18 -> He(33p) + He ................ C-120 -> He(43S) + He .............. C-122 -> He(43D) + He ................ C-122 -> He 4 He(43S) ................ C-124 -> He + He(43D) ................ C-]24 H+ + 51(2s) -> Li(2p) .................. _ • C-126 -> 5i(670,8 nra) .................. C-126 He+ + Li(2s) -> Li(670.8 nra) ................. C-128 He2+ _ Li(2s) -> bi(2p) ..................... C.-130 -> Li(670.8 nra) .................. C-130 D. Ionization Collisions and Charqe Production H '- H2 -> Total Slow Positive Ion Production ......... D-2 -> Total Slow Electron Production ............ D-2 -> H + H2. + e ...................... D-4 H/ + H -> H4 + H+ + e ...................... D-6 _|_ + H- -> H2+ + e ....................... D-J2 H+ t. H2 -->> THo.tal+ H2Slo•w e Elec.t.r.o.n......P.r.o.d.u.c.t.i.o.n. .......... DD--J!46 viii D. Ionization Collisions and Charqe Production (toni'd) O H* + H2 -> Total Production of H2+ ............... D-16 -> Total Production of H. ................ D-16 H. + He -> Electrons and H- . .................. D-18 -> H* + He* + e ......... D-24 -> (H + He*) or (H+ + He+ + e) .............. D-24 -> H+ + He2+ + 2e . . . . . ................ D-34 -> (H- + He2+) or (H* + He2* + 2e) ............ D-34 He(21S) + H -> He + H+ + e ................... D-42 -> He}l* + e ........... D'42 -> (He + H. + e) or Hell+ + e) ......... D-42 He(23S ) + H -> He + H+ + e ................... D-_4 -> Hell. + e ..................... D-44 -> (He + H* + e) or (Hell_ + e) ........... D-44 He(23S) + H2 -> Total Ionization ................ D-46 -> Rearrangement Ionization ............ D-46 He (21S) + H2 -> Total Ionization ................ D-48 -> Rearrangement Ionization ............ D-48 H* + He_ -> (H. + He2+ + e) .................. D-50 -> (H. + He2. + e) or (H° + He2+) ............ D-50 He. + He* -> (He. + Hez. + e) ......•...w..• • • • D-58 -> (He + He2_) or (He* + He2_ + e) .......... D-58 He + H2 -> Total Slow Positive Ion Production ......... D-64 -> Total Slow Electron Production ............ D-64 -> He + H2. + e ..................... D-66 -> Total H+ Production .................. D-66 He + He -> Total Slow Positive Ion Production .......... D-68 -> Total Slow Electron Production ............ D-68 -> He 4 He. + e ...................... D-70 -> He + He2* 4. ?e .................... D-70 He. _ H -> He+ + H. + e ..................... D-72 He. + H2 -> Total Slow Positive Ion Production ......... D-76 -> Total Slow Electrpn P_:oduction ........... D-76 He+ + H2 --> (He + H2.) or (He. + H2+ + e) ............ D-78 -> Total H. Production ................. D-78 -> He+ + H_ 4 H. + 2e ................. D-78 He. + He -> Total Slow Positive Ion Production ......... D-80 -> Total Slow Electron Production . , ......... D-80 I -> He* + He* + e ............... D-90 -> He+ + He2. + 2e . . . ................ D-90 He2_ + H -> He2. + H+ + e .................... D-96 He2+ + H2 -> Total Slow Positive ]on Production .......... D-]O0 -> Total Slow Electron Production ........... D-lO0 -> Total H. Production ................ D-lO2 -> H_ Production by Ionization Col]islons ....... D-102 -> Total tt2 Production ................ D-lO2 -> 1t2. Production by Single-Ionization ........ I)-.132 ix D. Ionizatlml ColllSious aild Charqe Production {Con t'd) He2. + He -> Total Slow Positive Ion Production ......... D-104 -> Total Slow Electron Productiol] ......... _ . . D-lO4 -> He2. + He+ + e ................... D-[I_ -> He2. + He2+ + 2e .................. D-II4 H+ + Li -> H. + Li+ i e . . . , . , . ....... . D-]22 He + + Li -> He_ + Li+ + e ................ .... D-126 He 2+ + Li -> He2. + Li_ + e ................... D-128 E. Electron Loss or Strippinq Collisions H + H -> H. + H + e ............ ........... E-2 H(2s) + H(Is) -> H+ + H 4 e ........ ..... ..... E-4 H + H2 -> H. + H2 + e ...................... E-6 H(28) + H2 -> H+ + H2 + e ................. .... E-8 H + He -> H. + He + e .................... E_]O H(2s) + He -> H. + He + e ...... ............. . F,-14 He + H -> He_ + H + e .................. E-16 He + H2 -> He. + H2 + e ..................... E-18 He + Hz -> He2. + Hz + 2e .................. , . B-J8 He* + H2 -> He or He+ ......... E-20 He* + H2 -> He_ + H2 + e ......... ........ . E-20 He* + H2 -> He + H2 .......... ........ E-2 o e O HHee •+ HHee -->> HHee+2+ ++HeHe ++ 2e ..................... EE--2222 He _ + H -> He2+ + H 4 e ...................... E-28 He . + H2 -> He2. + H2 + e ........ ............ E-30 He _ 4 He -> He_-. + He + e .................... E-32 F. Electron Detachment Collisions H- + H -> H + II + e ..................... F-2 -> (H + H + e) or (H + H-) ............... F-2 -> H+ _ H + 2e .................. F-4 11- + H_ -> H + H_ + 2e ............ . ........ F-6 H" + H2 -> H + H2 + e ...................... F-8 -> H+ + H2 + 2e ....................... F-10 H- + He -> H + He + e ...................... F-12 -> H+ + He + 2e ................... F-14 He" + H -> He + H + e ...................... F-16 He" + |I2 -> He + II2 + e ..................... F-18 -> He_ + H2 + 2e ........ . ............ F-18 He- + He -> He + He + e ................... F-20 -> He+ + He + 2e ................... F-20 Li" + H2 -> Li + H2 + e .................... F-22 -> Li+ + '_ + 2e F-22 Li" + He -> Li + He + e .................... F-24 -> Li+ } }le 4 2e .................... F-24 0 X , G. Dissociative Coli] sions H + H2 -> H-4 (H. 4 H*)+ e ................. 0-2 -> H + (H+ + H*) + 2e . • . ..... , , ...... 0-2 -> H+ -! (H_ + H+) + 3e .................... 0-2 -> H + (H + H_) 4 e . . • , ............ . . . 0-4 -> H+ + (li + H_) + 2e ............ . . . , . . . 0-6 -> lt- + (H' + H) ..... • • .............. C_-8 H* 4 li2 -> H+ + H+ + H+ _ 2e ................... , 0-].0 He+ + H2 -> He + + H . + H+ + 2e .... . . . ........... G-12 He2+ 4 H2 -> He2. + (H+ + H) + e (via iSOg) . .......... G-g4 -> He2. + (H . + H) 4 e (via 2POu) ..... ...... 6]-.16 .> He+ + (H. + HI • .................. O218 -> He+ + (H. + H ) + e . . ..... ......... 0-20 -> He2. + (H. + H.) + 2e ........ . . . . . . 0222 -> He + (H+ + H+) ' . .... ............... G-24 H2+ -_. H2 -5. H+proj. . ....................... G-26 H2+ + H -> H_proj. ....... ................... 0-28 H2. + H2 -> ||proJ. ................ ..... G-30 -> (H+ + H) + H2 ............... • .... 0-3.2 H2+ + He -> Total H+ • . • • ........ G-34 -> (H. + H) + He ........ ............ 0-36 O H2 + H2 -> H.(Fast,Total) .......... .......... G-38 -> H(Fast,To_al ) ................. 0-40 -> Total Destruction of Fast H2 Proj . . ........ G-42 H3 + + H2 -> Total Destruction of H3+ ....... .... 0-44 H2+ + H2 -> Total Destruction of H2+ . .............. 0-46 H3 + H2 -> H.(Total,Projectile) ................. 0-48 -> H2+ (Total, Projectile ) ................ 0-50 -> H(Total, Projectile) ................. G-52 -> H2(Total,Projectile) ................ . . G-54 H3_ + He -> H.(T0 tal) ................... . . . . G-56 -> H2 • • ..................... G-5R Hell . + H2 -> Total Hell . Disoociation Prod ............ G-60 HeH + + He -> Total HeH . Dissociation Prod. • .......... G-62 H, Particle Interchanqe Reactions H+ + D2 -> D+ + HD ....................... H-2 -> HD. + D ....................... H-2 HD+ + D2 -> HD2. + D ...... ................ H-4 -> D3+ + H ............. . ......... H-4 O

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